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According to The Sun, the veteran dance duo have been working on a track for the film themselves and are keen to get Winehouse involved.
"She’s got a few things to sort out first but we like her very much," said singer Neil Tennant.
"Technically she’s a great singer and we’ve got one or two tracks that would really suit her."
Mark Ronson revealed earlier this month that he had scrapped plans to work with Winehouse on a Bond theme because he wasn't sure she was "ready to work on music".
Pet Shop Boys confirmed last week that they would be teaming up with the pop production house Xenomania on a new album that will be released in 2009.
