The singer will include a rendition of the '80s group's classic hit 'Enjoy The Silence' on her upcoming LP Someone To Watch Over Me, reports The Sun.
The 50-year-old will also feature a cover of Tear For Fears hit 'Mad World' on the record, which is slated for a November 7 release.
Emeli Sandé has written some original material for the Britain's Got Talent finalist, who recently unveiled the album's trailer track 'You Have To Be There'.
Someone To Watch Over Me will be Boyle's third studio effort and follows her previous records I Dreamed A Dream and The Gift.
The star has managed to sell over 14 million albums worldwide since becoming an overnight YouTube sensation following the screening of her Britain's Got Talent audition in 2009.
> Susan Boyle reveals new album 'Someone To Watch Over Me' artwork
Watch the music video for Depeche Mode's 'Enjoy The Silence' below: