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The Quantum of Solace actress has co-written and sung a couple of tracks for the long-time Madonna collaborator.
The pair reportedly met backstage at a 2010 Madonna gig, and the Paris-based producer spent a year persuading the actress to work with him.
"I wrote text for him. He wrote music... and I kind of did the voice... for two songs - and I want to do more," she told Nylon magazine.
"It just comes out of me; I find the beauty in certain collisions of words. I didn't know how much passion was in music. Once you try it, you just want to do it all the time."
She added that her music career will likely remain a hobby, adding: "It's just a little thing."
Kurylenko recently signed up to star opposite Tom Cruise and Morgan Freeman in Joseph Kosinksi's untitled sci-fi project.
She will also appear with Woody Harrelson and Colin Farrell in Seven Psychopaths.
Watch the video for 'Naive Song' by Mirwais below:
