Connie Britton and Hayden Panettiere star in the series, which focuses on the careers of two country music stars.
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According to The Hollywood Reporter, the Fugees rapper will have a multiple episode arc on the first season of the show.
He posted a picture via his Twitter account featuring himself and co-stars Sam Palladio, Clare Bowen, Jonathan Jackson and Rya Kihlstedt.
Jean will reportedly play the head of a music label on the show, his first TV guest spot in two years.
The musician, activist and politician recently celebrated his 43rd birthday.
