Kebbel has appeared in several episodes of the show as Lexi, a vampire friend of Stefan (Paul Wesley) who was killed by Damon but reappeared as a ghost earlier this season.
Kebbel has now told TV Line that she would love the chance to appear on the show again.
"I would love, love, love to have Lexi pop up again," she said.
Kebbel also revealed that she would like to work with Joseph Morgan on the series, saying: "I'm looking forward to the day when Lexi gets to take on Klaus, but I don't know when that will be. I'm just determined to make that happen."
Kebbel, who has also starred in Gilmore Girls and Life Unexpected, is currently appearing as Vanessa in 90210.
The Vampire Diaries airs on Thursdays at 8/7c on The CW.